24 - Cobalt catalyst utility in organic synthesis

Description/Abstract/Artist Statement

Carbon-coupling reactions are important for the addition of new functional groups for biologically relevant molecules and in key intermediates for natural product synthesis. Such synthesis commonly utilizes transition metal catalysts such as palladium, indium, and ruthenium which are costly due to low environmental abundance. Therefore, exploration of cobalt catalysts are an optimal choice due to high abundances and thus environmental sustainability. Exploration of cobalt catalysts for organic synthesis, notably allylboration and prenylation reactions, have seen substantial conversion to the desired allyl and prenyl products via a Zimmerman-Traxler transition state. This method utilizes mild conditions as well as an aqueous solvent system. The development and mechanistic aspects of the methodology will be discussed.

Presenting Author Name/s

Olivia A Brown

Faculty Advisor/Mentor

Kyle M Lambert

Faculty Advisor/Mentor Department

Chemistry and Biochemistry

College Affiliation

College of Sciences

Presentation Type

Poster

Disciplines

Organic Chemistry

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24 - Cobalt catalyst utility in organic synthesis

Carbon-coupling reactions are important for the addition of new functional groups for biologically relevant molecules and in key intermediates for natural product synthesis. Such synthesis commonly utilizes transition metal catalysts such as palladium, indium, and ruthenium which are costly due to low environmental abundance. Therefore, exploration of cobalt catalysts are an optimal choice due to high abundances and thus environmental sustainability. Exploration of cobalt catalysts for organic synthesis, notably allylboration and prenylation reactions, have seen substantial conversion to the desired allyl and prenyl products via a Zimmerman-Traxler transition state. This method utilizes mild conditions as well as an aqueous solvent system. The development and mechanistic aspects of the methodology will be discussed.